extinction coefficient

Gary Hathaway (hathaway@cco.caltech.edu)
Sat, 11 Jul 1998 03:38:59 -0700

We've tried a Karl Fischer titration to measure water which was
subtracted

>from the overall lyophilized weight and still it came back high by
20%.

>I'm not sure if extraction with DMF before moisture analysis is able
to

>strip protein bound water off. Do you know?

>

>The counter-ion effect is something we are analyzing. We have
desalted the

>protein into H20 so the contribution of unbound salt is not there.
The Pi

>of the protein I believe is around 5 and the pH of the desalted
material

>into H20 is around 7. We've sent the protein for sodium analysis to

>analyze this counter-ion effect you mentioned.

>

>In you experience, what contribution weight does this counter ion
effect

>have vs. the bound H20 effect? Are we on the right path? Thank you
for

>your help. We will try to "dry" the protein down further.

>

>Best regards, John

John,


The effects of ion binding are very familiar to physical chemists who
do things like trying to interpret the distribution of proteins in
centrifugal fields in terms of molecular weight. In that case, the
difference between bound solvent + ions and bulk solvent can have a
significant effect due to buoyancy. In the case of the extinction
coefficient, the weight of the (assumed) protein may vary depending on
the extent of interaction with solutes, so it's hard to predict which
will have the greater effect. Have you considered doing AAA for weight?
The accuracy for determining the <italic>amount of protein</italic> is
much higher than compositional error. By summing the pmoles of amino
acids you should get to 95%+ accuracy and this is independent of the
presence of bound counterions as it involves no weighing.

regards

--------------------------------------------------

Gary M. Hathaway, Director

PPMAL - Protein/Peptide Micro Analytical Laboratory

California Institute of Technology

139-74, Division of Biology

Pasadena, CA 91125

http://www.cco.caltech.edu/~ppmal

email Gary: hathaway@cco.caltech.edu

email facility: ppmal@cco.caltech.edu

phone: lab (626) 395-6388 or office (626) 395-2769

FAX (626) 449-3414

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